Let f1 be the fraction of isotope 1 and f2 be the fraction of isotope 2. Then:
f1 + f2 = 1
68.926*f1 + 70.925*f2 = 69.72
Replace f2 in the second equation using the fact that f2 = 1 - f1 from the first equation and solve for f1:
$${\mathtt{68.926}}{\mathtt{\,\times\,}}{\mathtt{f1}}{\mathtt{\,\small\textbf+\,}}{\mathtt{70.925}}{\mathtt{\,\times\,}}\left({\mathtt{1}}{\mathtt{\,-\,}}{\mathtt{f1}}\right) = {\mathtt{69.72}} \Rightarrow {\mathtt{f1}} = {\frac{{\mathtt{1\,205}}}{{\mathtt{1\,999}}}} \Rightarrow {\mathtt{f1}} = {\mathtt{0.602\: \!801\: \!400\: \!700\: \!350\: \!2}}$$
So f1 ≈ 0.603 and f2 ≈ 1 - 0.603 = 0.397
or f1 ≈ 60.3% and f2 ≈ 39.7%
.